The new possibilities for use of artificial intellect methods in atmospheric researches are described. The results of three wavelengths fuzzy ozonometer are discussed. The well-known Dobson method of total ozone measurements is realized using fuzzy logic method.The principles of development of fuzzy controller are formulated. The new method for multicriterial optimization of measuring systems is developed. The method provides for joint optimization of of partial criteria used for crisp and fuzzy systems.The variation optimization method is used for development of effective system for control of atmosphere. The questions on optimal development of local ozonometric network are considered. The analysis of existing models for propagation of atmospheric aerosol is given. Optimization of airborne video complex operating in multiple measuring regime is carried out.